荷电水雾团聚亚微米颗粒物试验研究Experimental investigation on submicron particle agglomeration through atomized charged droplets
刘鹤欣,杨富鑫,李正鸿,谭厚章,杜勇乐,冯鹏
LIU Hexin,YANG Fuxin,LI Zhenghong,TAN Houzhang,DU Yongle,FENG Peng
摘要(Abstract):
荷电水雾团聚亚微米颗粒物是多场协同脱除微细颗粒物的一种方式,众多学者针对水雾荷电脱除颗粒物特性进行了大量理论和试验研究,但鲜见对超声波雾化液滴荷电团聚微细颗粒物的相关研究。设计了双层阻挡介质放电电极结构,在有效阻断传统电晕放电隙内放电电弧发展的同时,通过产生均匀稳定的高密度低温等离子体对雾化液滴进行荷电,并搭建荷电水雾团聚亚微米颗粒物试验平台对电极稳定特性和微细颗粒物的团聚特性进行研究,主要针对电极伏安特性、负载电压对团聚效率的影响以及水雾量对团聚效率的影响3方面进行比较与表征。结果表明,双层阻挡介质结构有利于改善荷电电极间隙的均匀性,雾化液滴的存在有利于促进气隙空间放电。荷电电极的起晕电压与不稳定运行电压随雾化量的增加均表现为减小;当通入水雾流量为102.9 mg/min时,稳定运行的电压区间为17.2~41.1 kV。荷电雾化液滴对微细颗粒物团聚具有明显效果,其中30~70 nm颗粒在45.0 kV作用下最高达到40%团聚效率。粒径分布曲线随雾化量的增加整体向粒径增大方向移动,也表明雾化量的增加有利于荷电雾化液滴对微细颗粒物的脱除;相同电压下,颗粒团聚效果随水雾量的增加明显提升。
The submicron particle agglomeration by atomized charged droplets is an effective method of multi-field synergistic agglomeration of fine particles. Many scholars have carried out a lot of theoretical and experimental studies on the characteristic of fine particle removal through charged droplets. However,few studies have been conducted on the study of fine particle agglomeration of atomized charged droplets with particle size diameter of about 5 μm. In this paper,a double-layer dielectric barrier discharge electrode was designed to effectively block the development of the discharge arc in the traditional corona discharge gap and charge the atomized droplets by producing a uniform and stable high-density low-temperature plasma. Meanwhile,an experimental platform of submicron particle agglomeration through the atomized charged droplets was built for the experimental study of electrode stability and agglomeration characteristics of fine particles. Three aspects of electrode volt-ampere characteristics,the influence of load voltage on the agglomeration efficiency,and the influence of water mist quantity on the agglomeration efficiency were compared and characterized. The results show that the structure of the double-layer barrier medium is beneficial to improve the uniformity of the gap between charged electrodes,and the existence of atomized droplets is beneficial to promote the discharge in air gap space. Both the initiation voltage and unstable operating voltage of charged electrode decrease with the increase of the water mist flow. When the water mist flow is 102.9 mg/min,the voltage range for stable operation is17.2-41.1 kV. The atomized charged droplets have obvious effect on the agglomeration of fine particles. The agglomeration efficiency of 30-70 nm particles can reach up to 40% under the action of 45.0 kV. With the increase of atomization amount,the particle size distribution curve moves towards the increase of particle size as a whole,which also indicates that the increase of atomization amount is conducive to the removal of fine particles by charged atomization droplets. Under the condition of the same voltage,the particle agglomeration effect is significantly improved with the increase of the water mist flow.
关键词(KeyWords):
超声波雾化荷电;介质阻挡放电;团聚效率;亚微米颗粒;伏安特性
ultrasonic atomizing charge;dielectric barrier discharge;agglomeration efficiency;submicron particles;Volt-ampere characteristic
基金项目(Foundation): 国家重点研发计划资助项目(2016YFB0601504)
作者(Author):
刘鹤欣,杨富鑫,李正鸿,谭厚章,杜勇乐,冯鹏
LIU Hexin,YANG Fuxin,LI Zhenghong,TAN Houzhang,DU Yongle,FENG Peng
DOI: 10.13226/j.issn.1006-6772.IF20080617
参考文献(References):
- [1]LEAR C W,KRIEVE W F,COHEN E.Charged droplet scrubbing for fine particle control[J].Journal of the Air Pollution Control Association,1975,25(2):184-189.
- [2]METZLER P,WEIP,BTTNER H,et al.Electrostatic enhancement of dust separation in a nozzle scrubber[J].Journal of Electrostatics,1997,42(1/2):123-141.
- [3]D'ADDIO L,DI NATALE F,CAROTENUTO C,et al.A lab-scale system to study submicron particles removal in wet electrostatic scrubbers[J].Chemical Engineering Science,2013,97:176-185.
- [4]CAROTENUTO C,NATALE F D,LANCIA A.Wet electrostatic scrubbers for the abatement of submicronic particulate[J].Chemical Engineering Journal,2010,165(1):35-45.
- [5]BALACHANDRAN W,KRUPA A,MACHOWSKI W,et al.Smoke precipitation by charged water aerosol[J].Journal of Electrostatics,2001,51(1):193-199.
- [6]BALACHANDRAN W,JAWOREK A,KRUPA A,et al.Efficiency of smoke removal by charged water droplets[J].Journal of Electrostatics,2003,58(3):209-220.
- [7]LAW S.Charge and mass flux in the radial electric field of an evaporating charged water droplet:An experimental analysis[J].IEEE Transactions on Industry Applications,1989,25 (6):1081-1087.
- [8]POLAT M,POLAT H,CHANDER S,et al.Characterization ofairborne particles and droplets[J].Particle&Particle Systems Characterization,2015,19(1):38-46.
- [9]吴琨,王京刚,毛益平,等.荷电水雾振弦除尘器的性能研究[J].有色金属(矿山部分),2004,56(5):46-48.WU Kun,WANG Jinggang,MAO Yiping,et al.Research on the performance of the charged spray vibratin string dust collector[J].Nonferrous Metals(Mining Section),2004,56(5):46-48.
- [10]吴琨,王京刚,毛益平,等.荷电水雾振弦栅除尘技术机理研究[J].金属矿山,2004,56(8):59-62.WU Kun,WANG Jinggang,MAO Yiping,et al.Study on mechanism of vibrating grid dedusting technology with charged fog[J].Metal Mine,2004,56(8):59-62.
- [11]陈卓楷,陈凡植,周炜煌,等.超声雾化水雾在除尘试验中的应用[J].广东化工,2006,33(10):74-77.CHEN Zhuokai,CHEN Fanzhi,ZHOU Weihuang,et al.The application of atomization water made by ultrasonic technique in dust removal experiment[J].Guangdong Chemical Industry,2006,33(10):74-77.
- [12]马素平,寇子明.喷雾降尘机理的研究[J].煤炭学报,2005,30(3):297-300.MA Suping,KOU Ziming.Study on mechanism of reducing dust by spray[J].Journal of China Coal Society,2005,30 (3):297-300.
- [13]左子文.荷电液滴捕集颗粒物机理和特性的研究[D].镇江:江苏大学,2016.ZUO Ziwen.Research on the mechanism and characteristics of charged droplets to capture particles[D].Zhenjiang:Jiangsu University,2016.
- [14]ANTES T,SZUDYGA M,LIWI SKI,et al.Future needs for ship emission abatement and technical measures[J].Transport Problems An International Scientific Journal,2013,8(3):101-107.
- [15]HA T H,NISHIDA O,FUJITA H,et al.Enhancement of diesel particulate matter collection in an electrostatic water-spraying scrubber[J].Journal of Marine Science&Technology,2010,15(3):271-279.
- [16]SUN Yanzhou,QIU Yuchang,YU Fashan,et al.Application of DBD and DBCD in SO2removal[J].Plasma Science and Technology,2004,6(6):2589-2592.
- 超声波雾化荷电
- 介质阻挡放电
- 团聚效率
- 亚微米颗粒
- 伏安特性
ultrasonic atomizing charge - dielectric barrier discharge
- agglomeration efficiency
- submicron particles
- Volt-ampere characteristic